Atmospheric Reactive Nitrogen Cycle and Stable Nitrogen Isotope Processes: Progresses and Perspectives   总被引：1，自引：1，他引：0  

Tao Zhou  Zhuang Jiang  Lei Geng 《地球科学进展》2019,34(9):922-935

Oxidized reactive nitrogen in the atmosphere mainly consists of nitrogen oxides (NO _X =NO+NO₂, NO₃) and nitric acid. The atmospheric cycling of NO _X influences the formation of ozone and hydroxyl radicals that are important for atmospheric oxidation capacity. Nitric acid, the final product of NO _X oxidation, not only is an important component of particulate pollutants, but also has a direct impact on the ecosystem through dry and wet deposition. The stable nitrogen isotope (δ¹⁵N) shows the potential to study reactive nitrogen cycle, and to trace the emission, transport and deposition of reactive nitrogen from local to global scales. Here, we reviewed previous studies using δ¹⁵N to investigate NO _X emission and atmospheric reactive nitrogen cycle, and discuss the uncertainties of δ¹⁵N signatures of different NO _X sources from two aspects: NO _X generation mechanism and NO _X collection methods. We also discussed the nitrogen isotope fractionation and the consequences during the conversions of NO _y molecules. We ended up with discussions on the possibility of using δ¹⁵N to trace NO _X emissions. Although there are still large uncertainties in quantifying and tracing NO _X emissions using nitrogen stable isotopes, such isotope tool is efficient enough to trace reactive nitrogen cycles in the atmosphere. On the basis of this, we proposed that we can combine atmospheric chemistry transmission models with isotope tracers to improve our understanding of regional and global atmospheric reactive nitrogen cycle regarding the fluxes of different emission sources, their atmospheric transformation, etc.  相似文献   

大连市大气污染物质量浓度与气溶胶光学厚度的相关性分析     

顾吉林  汤宏山  刘淼  耿杨  于月  陶涛 《地理科学》2019,39(3):516-523

分别对2015年6~12月和2016年6~12月大连地区的大气污染物PM2.5、PM10、SO₂、NO₂、CO和O₃的浓度数据进行数据统计分析,基于ENVI软件平台利用MODIS数据反演大连地区的气溶胶光学厚度,通过回归建模研究气溶胶光学厚度与大连地区10个地面监测站点的大气污染物PM2.5、PM10、SO₂、NO₂、CO和O₃的浓度数据的相关性。回归建模以气溶胶光学厚度（AOD）为自变量,以大气污染物PM2.5、PM10、SO₂、NO₂、CO和O₃为因变量,在SPSS软件中分别选取线性、对数、三次、乘幂、指数5种函数类型进行研究,通过对比回归模型的拟合优度R²,选择最优拟合模型,探讨利用遥感数据反演气溶胶光学厚度监测大气污染的相关性。结果表明：气溶胶光学厚度与NO₂、PM2.5和PM10的最优拟合模型均为三次模型,其拟合优度R²分别是0.685、0.801和0.845;与O₃和SO₂的最优拟合模型为指数模型,其R²为0.367和0.482;与CO的最优拟合模型为对数模型,其拟合优度R²为0.810。该结果为分析大气气溶胶污染来源以及治理提供了数据。  相似文献   

超慢速扩张环境下超镁铁质岩系统的热液硫化物成矿机理以及启示     

曹红  孙治雷  刘昌岭  姜学钧  何拥军  黄威  尚鲁宁  王利波  张喜林  耿威  施美娟  李东义 《海洋学报》2018,40(4):61-75

西南印度洋63.5°E热液区是在超慢速扩张洋脊发现的首个超镁铁质岩热液系统。对取自该区的热液硫化物样品进行了系统的矿物学和地球化学分析，矿物学分析结果表明:该热液区硫化物为富Fe型高温硫化物，且经历了较深程度的氧化蚀变，大量中间态的Fe氧化物充填在硫化物矿物间的孔隙及内部解理中；这些硫化物相以白铁矿为主，其次是等轴古巴矿和少量铜蓝，缺乏黄铁矿、闪锌矿。据推断，该区的热液成矿作用分为4个阶段:低温白铁矿阶段→高温等轴古巴矿阶段→自形白铁矿阶段→后期海底风化阶段（少量铜蓝以及大量的Fe的羟氧化物）。与之相对应，地球化学分析结果表明这些硫化物的Fe含量较高（31.57%~44.59%），Cu含量次之（0.16%~7.24%），而Zn含量普遍较低（0.01%~0.11%）；微量元素较为富集Co（328×10-6~2 400×10-6）和Mn（48.5×10-6~1 730×10-6）。该区硫化物中较高含量的Fe、Co与超镁铁质岩热液系统相似，明显高于镁铁质岩热液系统。独特的热液硫化物矿物学特征和元素组成可能与该区普遍出露的地幔岩、橄榄岩蛇纹石化作用以及拆离断层的广泛发育的环境有关。  相似文献   

A model of fast radio bursts: collisions between episodic magnetic blobs     

Long-Biao Li  Yong-Feng Huang  Jin-Jun Geng  Bing Li 《天文和天体物理学研究(英文版)》2018,(6)

Fast radio bursts(FRBs) are bright radio pulses from the sky with millisecond durations and Jansky-level flux densities. Their origins are still largely uncertain. Here we suggest a new model for FRBs. We argue that the collision of a white dwarf with a black hole can generate a transient accretion disk, from which powerful episodic magnetic blobs will be launched. The collision between two consecutive magnetic blobs can result in a catastrophic magnetic reconnection, which releases a large amount of free magnetic energy and forms a forward shock. The shock propagates through the cold magnetized plasma within the blob in the collision region, radiating through the synchrotron maser mechanism,which is responsible for a non-repeating FRB signal. Our calculations show that the theoretical energetics, radiation frequency, duration timescale and event rate can be very consistent with the observational characteristics of FRBs.  相似文献   

Effect of sand on the vacuum consolidation of dredged slurry     

Jun Wang  Yuanqiang Cai  Xueyu Geng  Fengqi Xu 《Marine Georesources & Geotechnology》2018,36(2):238-244

Vacuum preloading is often used to improve the geotechnical properties of dredged slurry. Although the performance of this method has improved with rapidly developing technology, soil columns usually formed on the drainage boundary induce the decrease of permeability around the boundary, thereby limiting the further development of this method. To address this issue, this paper proposes a method for pretreating the slurry combined with sand prior to vacuum consolidation. This method partially replaces the fine particles with sand to reduce the formation of soil columns. Two groups of vacuum preloading tests were performed to investigate the effect of sand content and sand grain size on the vacuum consolidation of dredged slurry. The test results revealed that for a given sand grain size, increasing the sand content of the sand–slurry mixture increased the pore water drainage and accelerated the dissipation of pore water pressure, thereby increasing the vane shear strength. In contrast, for a constant sand content, the samples containing coarse sand exhibited increased pore water drainage and accelerated dissipation of pore water pressure, thereby increasing the vane shear strength of the soil.  相似文献   

Hydroacoustic estimates of fish biomass and spatial distributions in shallow lakes     

连玉喜  黄耿  Ma?gorzata GODLEWSKA  蔡杏伟  李昌  叶少文  刘家寿  李钟杰 《中国海洋湖沼学报》2018,36(2):587-597

We conducted acoustical surveys with a horizontal beam transducer to detect fish and with a vertical beam transducer to detect depth and macrophytes in two typical shallow lakes along the middle and lower reaches of the Changjiang(Yangtze) River in November 2013. Both lakes are subject to active fish management with annual stocking and removal of large fish. The purpose of the study was to compare hydroacoustic horizontal beam estimates with fish landings. The preliminary results show that the fish distribution patterns dif fered in the two lakes and were af fected by water depth and macrophyte coverage. The hydroacoustically estimated fish biomass matched the commercial catch very well in Niushan Lake, but it was two times higher in Kuilei Lake. However, acoustic estimates included all fish, whereas the catch included only fish 45 cm(smaller ones were released). We were unable to determine the proper regression between acoustic target strength and fish length for the dominant fish species in the two lakes.  相似文献   

华南桉树人工林芒萁层片的生态筛效应     

刘美洁  孙中宇  耿守保  温美丽  戴佳玲  杨龙 《热带地理》2021,41(6):1338-1346

芒萁是华南退化坡地上最具代表性的先锋种、优势种和关键种,能够快速形成密集的单优种层片结构。与传统阻碍更新的观点不同,野外观察发现芒萁层片内仍有少数物种能够成功定居,被认为具有生态筛效应。文章通过设置4种芒萁层片处理（芒萁层片完全剔除-UR;仅保留地上层-AF;仅保留根毯层-AR;芒萁层片全部保留-CK）,分别在不同处理下移植目标种幼苗并结合土壤性状,探究芒萁层片生态筛效应及其潜在机理。结果发现：1）桉林芒萁根毯层中土壤有机质、全氮、碱解氮、有效磷、速效钾、交换性钠、交换性钙、交换性镁和阳离子交换量均显著高于芒萁红壤层和裸地红壤;2）多数乔木种和草本种在芒萁根毯层保留时无法存活,仅荷木、桃金娘、梅叶冬青和野牡丹等目标种幼苗在保留芒萁根毯层处理（AR和CK）下能够存活与生长。这表明芒萁层片确实具有生态筛效应,且其关键在于根毯层的作用而并非土壤养分改善作用。理论上,芒萁层片（尤其是根毯层）与生态恢复的生物阈值突破密切相关,未来需要进一步解析芒萁根毯层的结构与功能。应用上,华南地区存在大量以芒萁为单优林下植物的人工林类型（如桉林等）,在进行结构优化与林分改造时需注意芒萁的生态筛效应。  相似文献   

Improving BDS integer ambiguity resolution using satellite-induced code bias correction for precise orbit determination     

Geng  Tao  Xie  Xin  Zhao  Qile  Liu  Xianglin  Liu  Jingnan 《GPS Solutions》2017,21(3):1191-1201

GPS Solutions - Successful resolution of integer ambiguity over long baselines is a key to improve the accuracy of precise orbit determination for global navigation satellite system satellites. The...  相似文献   

东北亚地区M_S6.0以上地震异常电磁波动研究     

杨牧萍  钱庚  张学民  申旭辉  张萌  金艳铭 《大地测量与地球动力学》2022,42(7):669-674

利用2005-01~2009-12 DEMETER电磁卫星详查模式下磁场与电场的极低频（ELF）三分量波形数据,选取东北亚地区（38°~58°N,105°~145°E）6个M_S≥6地震,对震前30 d震中上空±10°的6 000余条1130和1135轨道数据进行波矢分析和坡印廷矢量分析。结果发现,2005-08-16日本本洲东岸近海M_S7.2地震和2009-06-05日本北海道地区M_S6.6地震震前在质子回旋频率以下记录到来源于地球的异常电磁波扰动;2005-11-10俄罗斯西伯利亚东南部M_S6.4地震和2007-08-02俄罗斯萨哈林岛(库页岛)M_S6.8地震震前在质子回旋频率以下没有记录到异常电磁波扰动;2007-02-17日本北海道地区M_S6.2地震和2008-06-13日本本州东岸近海M_S7.3地震震前在质子回旋频率以下记录到异常电磁波扰动,但并非来源于地球。  相似文献   

扬子克拉通北缘中元古界神农架群沉积特征^*          下载免费PDF全文

旷红伟  柳永清  范正秀  彭楠  耿元生  朱志才  许欢  安伟  王能盛  夏晓旭  王玉冲 《古地理学报》2018,20(4):523-544

神农架群(约1400—1000 Ma)发育于扬子克拉通北缘鄂西北地区,自下而上发育有下亚群(大岩坪组、马槽园组、乱石沟组、大窝坑组和矿石山组)、中亚群(台子组、野马河组、温水河组和石槽河组)及上亚群(送子园组和瓦岗溪组)。每亚群均由相对较深水相碎屑岩和浅水碳酸盐岩组成。一系列岩石组合特征、宏微观沉积组构和沉积构造等表明,神农架群发育环潮坪相藻碳酸盐岩、浅海相碎屑岩、台缘浅滩颗粒碳酸盐岩和台缘斜坡砾屑碳酸盐岩等4类沉积组合,形成于远端变陡型缓坡型碳酸盐岩台地背景。环潮坪沉积分布最广,遍布于所有碳酸盐岩地层,不同类型叠层石发育,构成向上变浅沉积序列;进积作用强烈,干裂构造、蒸发岩等常见;沉积相带由浅潮下、潮坪及潮上带组成。浅海碎屑岩沉积组合主要见于台子组及大岩坪组,由砂岩、粉砂岩与泥岩组成,石英砂岩分选和磨圆较好,自生海绿石常见,平行层理、水平—波状层理发育,泥岩中自生黄铁矿发育,总体经历了滨岸浅滩—浅海陆棚—碎屑潮坪—局限台地等的高频变化。台缘浅滩颗粒碳酸盐岩以鲕粒白云岩、砾屑白云岩(及内碎屑白云岩)和斜歪锥、柱状叠层石为特征,主要见于乱石沟组、野马河组;大窝坑组及石槽河组以鲕粒和砂—砾屑白云岩及藻碎屑(团块或凝块石)为特征;大中型板状交错层理、递变—平行层理和冲刷—侵蚀构造普遍,表明浅潮下带强水动力条件环境。台缘斜坡砾屑碳酸盐岩发育在大岩坪组中上部及马槽园组,由滑塌堆积的透镜状、巨厚层状巨—粗—细砾岩和砂岩组成,砾岩成分以白云岩等为主,可见大型交错层理、波痕和侵蚀—冲刷等沉积构造。对神农架群沉积序列、沉积特征及沉积演化过程的研究,为扬子克拉通中元古代晚期的盆地演化与重建、沉积充填过程及地层—沉积对比研究提供了基础资料及依据。  相似文献